Cryogenic signal amplification combined with helium-temperature MAS DNP toward ultimate NMR sensitivity at high field conditions #DNPNMR

Published: Friday, 01 April 2022 - 00:00 UTC

Author: Thorsten Maly

Matsuki, Yoh, Shinji Nakamura, Fumio Hobo, Yuki Endo, Hiroki Takahashi, Hiroto Suematsu, and Toshimichi Fujiwara. “Cryogenic Signal Amplification Combined with Helium-Temperature MAS DNP toward Ultimate NMR Sensitivity at High Field Conditions.” Journal of Magnetic Resonance 335 (February 2022): 107139.

https://doi.org/10.1016/j.jmr.2021.107139.

The low sensitivity of NMR spectroscopy is of historical concern in the field, and various approaches have been developed to mitigate this limitation. On the shoulder of giants, today one can routinely implement, for example, the pulse/Fourier transform NMR with the cross polarization together with the ultra-low temperature MAS DNP under high-field conditions. We show in this work this current opportunity should further be augmented by combining them with the cryogenic signal amplification. Our presented MAS DNP probe operates with the closed-cycle helium MAS system, and cools the internal preamplifierduplexer module with the ‘‘return” helium gas on its way back to the compressor in the loop. The signal-to-noise (S/N) gain relative to the room-temperature measurements of a factor of 4.6 and 2.4 was found for the measurement using the cold- and room-temperature preamplifier, respectively, at the sample temperature of T = 20 K at B0 = 16.4 T. The ratio of these factors reveals $ two-fold sensitivity improvement that results purely from the introduction of the cold signal amplification, i.e., noise reduction. Together with the increase of the thermal Boltzmann polarization at low temperatures, the combined S/N gain of max. $70-fold is possible without DNP. The DNP enhancement factor of $40 as we found in this work for a microcrystalline MLF sample may be multiplied to this gain. We also demonstrated the sensitivity improvement with a 13C-detected 2D NCaCx spectrum, illustrating the generality of the S/N gain from combining DNP with the cold signal amplification.